Abstract
We investigate the effects of magnetic impurities on the upper critical field (μ 0 H c2) in La-doped CaFe2As2 (LaCa122) single crystals. The magnetic field dependency of the superconducting transition temperature (T c) for LaCa122 is rapidly suppressed at low fields up to ~1 kOe despite its large μ 0 H c2(0) value on the order of tens of Tesla, resulting in a large positive curvature of μ 0 H c2(T) near T c. The magnetization hysteresis (M–H) loop at temperatures above T c shows a ferromagnetic-like signal and the M(H) value rapidly increases with increasing magnetic field up to ~1 kOe. Taken together with the linear suppression of T c with the magnetization in the normal state, these results suggest that the large upward curvature of μ 0 H c2(T) near T c in La-doped CaFe2As2 mainly originates from the suppression of superconductivity due to the presence of magnetic impurities.
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