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Nye ligander for Pt-MOF strukturer

Jakobsen, Søren
Master thesis
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soren_jakobsen_small.pdf (21.74Mb)
Year
2006
Permanent link
http://urn.nb.no/URN:NBN:no-12651

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  • Kjemisk institutt [843]
Abstract
Metalorganic frameworks (MOFs) are a new type of compounds which have been intensely investigated during the last few years. They have been synthesized using a wide variety of metals and ligands constructing a vast number of 1, 2 and 3 dimensional structures, some of which possess zeolite-type physics and chemistry.

Our approach is to incorporate platinum metal sites into the structures making them bimetallic and potentially catalytically active. Therefore a number of N-N-type ligands (diimines, phenanthrolines and bipyridines) and their dichloro-platinum complexes have been prepared and used as linkers in MOF synthesis.

To make the chemistry and ideas of MOFs understandable to chemists on all levels, a comprehensive theoretical part considering homogeneous catalysis, heterogeneous catalysis, MOFs in general, heterocyclic chemistry and characterization techniques has been included.

The thesis is written in Danish.

Keywords: Pt, platinum, platina, ligand, complex, komplex, MOF, metalorganic framework, coordination polymer, koordinasjons polymer.
 
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